The Priest Tier 5. Avatar Regalia. http://www.wowhead.com/itemset=665#. I LOVED that set from the moment I saw it. Made me think of Tyrael from Diablo and I aspired to get it. It has become my characters "everyday" outfit if I'm not questing or running an instance. I probably never woulda made a priest without that set being out. Again I tell you, Priest Tier 5. For the Light!
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Having started in The Burning Crusade I would have to say Tier 4 and more specifically the Hunter Demonstalker gear would be my favorite set. I think the reason I like it so much is that it was my first set to look forward to. I was ecstatic to have finally hit level 70 and see that there are such cool sets of gear that i could obtain. At the time the world was still so fresh and new to me that every new piece of gear was something to be proud of.
t6 set, the concept of the tier almost represent the class itself.
Seeing as I play a shaman, my favourite was back in the short-lived Ulduar patch.Conqueror's Worldbreaker. The shoulderpads are absolutely beautiful.However, if they made an itemset out of the new ZA/ZG gear for shamans, I would definitely choose that. But alas, they are not part of an itemset.
I would have to say Tier 10, because I started playing around the release of 3.3 and it was the first set I completed and felt good about :DUntil I found out everyone else had a whole set.
I really liked the Ymirjar Lords plate because it was the first complete set I had that looked really cool together.
My Favourite Tiear set even though my main is a hunter, it has to be the Priest Tier 3, i always loved that set and the recoloured tier 7 was nice, but the tier 3 was just my favourite tier ever. ow how i miss tier 3:(
I would have to say that the tier 6 shaman set Skyshatter Raiment is by far my favorite set. As a diehard shaman I believe it to be the best looking shaman set ever and it was the set that was around during a time when resto shamans were the healing kings(and queens).
My favorite is the Paladin tier 2 armor, Judgement. Everything about it is so epic; the name, the look, the colors... It just looked so paladin. It actually inspired me to play WoW, I saw it looking through wowhead one day deciding whether to buy the game or not when I came across it, instantly I said "I'm buying the game and getting that set." Cheers Blizzard/wowhead.
I'd have to go with the Druid Tier 5 Balance set Nordrassil Regalia This set was great for running as a hybrid as the 2 piece bonus was great for shifting to a healer role out of damage, and the 4 piece bonus was a nice little boost in straight dps!